Park, Sohyun published the artcileValidating the Mott Formula with Self-Assembled Monolayer (SAM)-Based Large-Area Junctions: Effect of Length, Backbone, Spacer, Substituent, and Electrode on the Thermopower of SAMs, Formula: C8H10S, the publication is Journal of Physical Chemistry C (2021), 125(36), 20035-20047, database is CAplus.
Understanding how the Seebeck effect of organic thermoelec. devices is associated with the chem. structure of active mols. within the devices is a key goal in organic and mol. thermoelecs. This paper describes a series of phys.-organic studies that investigate structure-thermopower relationships in self-assembled monolayers (SAMs) through measurements of the Seebeck coefficient (S, μV/K) using the eutectic gallium-indium (EGaIn)-based junction technique. Several hypotheses were derived from a transmission function-based simple toy model, the Lorentzian transmission function-based Mott formula. These hypotheses were tested by comparing values of S for simple alkyl and aryl mols. with different structures in terms of backbone, length, spacer, anchor, and substituent, and for different electrodes (Au vs Ag), and by monitoring responses of S to the structural modifications. Exptl. obtained S values were further reconciled with values simulated by the Mott formula and with interfacial electronic structure and mol.-electrode coupling strength, independently measured by UPS and transition voltage spectroscopy.
Journal of Physical Chemistry C published new progress about 4410-99-5. 4410-99-5 belongs to alcohols-buliding-blocks, auxiliary class Thiol,Benzene, name is 2-Phenylethanethiol, and the molecular formula is C8H10S, Formula: C8H10S.
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